Source code for PDielec.Materials

#
# Copyright 2024 John Kendrick & Andrew Burnett
#
# This file is part of PDielec
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# This program is free software; you can redistribute it and/or modify
# it under the terms of the MIT License
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"""Materials DataBase.

An interface to the spreadsheet which holds materials data
"""

import logging
import math
import os
import warnings

import numpy as np
import openpyxl as xl

import PDielec
from PDielec import Calculator, DielectricFunction
from PDielec.UnitCell import UnitCell

logger = logging.getLogger(__name__)



[docs] class MaterialsDataBase: """A class for managing a database of materials' properties. This database is initialized from an Excel spreadsheet which contains various material properties including names, densities, refractive indices, and permittivities, among others. Additional functionalities include validation checks, retrieval of sheet names, material information, and specific data based on the property of interest (e.g., constant permittivity, tabulated refractive index). The get_material() method returns a material with a dielectric function of the appropriate type. There are routines which read (process) the data stored for the following dielectric functions: - constant refractive index - constant permittivity - tabulated refractive index (may be 1, 3 or 6 parameters for isotropic, uniaxial or anisotropic) - tabulated permittivity (may be 1, 3 or 6 parameters for isotropic, uniaxial or anisotropic) - Lorentz-Drude - FPSQ (Four parameters semi-quantum model) - Sellmeier Further information can be found in the following classes and their sub-classes: - :class:`~PDielec.Materials.Material` - :class:`~PDielec.DielectricFunction.DielectricFunction` Parameters ---------- filename : str The filename of the spreadsheet/database. debug : bool, optional Set to true for additional debugging information Attributes ---------- filename : str The path to the Excel spreadsheet containing materials data. sheetNames : list A list of strings representing the names of the sheets within the Excel spreadsheet. cache : dictionary A dictionary of materials that have been read from the database debug : bool, optional A flag indicating whether debugging information should be printed. Default is False. Methods ------- __init__(filename, debug=False) Initializes the MaterialsDataBase class with a given Excel spreadsheet and a debug flag. get_file_name() Returns the filename of the Excel spreadsheet being used as the database. valid() Checks if the spreadsheet is a valid materials database based on certain criteria. get_sheet_names() Retrieves a sorted list of sheet names within the spreadsheet, including additional predefined names. get_material(sheet) Returns a material object based on the data in a given sheet of the Excel spreadsheet. read_constant_refractive_index(sheet, worksheet, density) Reads constant refractive index data for a given material from the spreadsheet. read_constant_permittivity(sheet, worksheet, density) Reads constant permittivity data for a given material from the spreadsheet. read_tabulated_refractive_index(sheet, worksheet, density) Reads tabulated refractive index data for a given material from the spreadsheet. read_tabulated_spectroscopy(sheet, worksheet, density) Reads tabulated n and alpha (in cm-1) data for a given material from the spreadsheet. read_tabulated_permittivity(sheet, worksheet, density) Reads tabulated permittivity data for a given material from the spreadsheet. read_lorentz_drude(sheet, worksheet, density, unitCell) Reads Drude-Lorentz model parameters for a given material from the spreadsheet. read_fpsq(sheet, worksheet, density, unitCell) Reads FPSQ model parameters for a given material from the spreadsheet. read_sellmeier(sheet, worksheet, density, unitCell) Reads Sellmeier model parameters for a given material from the spreadsheet. """ def __init__(self,filename, debug=False): """Initialise a database of material properties using the excel spreadsheet filename. Parameters ---------- filename : str The filename of the spreadsheet/database. debug : bool, optional Set to true for additional debugging information """ logger.debug("Start:: initialise") if len(filename)> 5 and (filename.endswith("xlsx") or filename.endswith("XLSX")) and os.path.isfile(filename): self.filename = os.path.relpath(filename) with warnings.catch_warnings(): warnings.filterwarnings("ignore", "Workbook contains no default style", UserWarning) self.workbook = xl.load_workbook(self.filename,data_only=True) self.sheetNames = self.workbook.sheetnames logger.debug(f"Sheet names:: {self.sheetNames}") # Close the work book while it is not in use # workbook.close() else: # Try opening the default database PDielec_Directory = os.path.dirname(PDielec.__file__) filename = os.path.join(PDielec_Directory, "MaterialsDataBase.xlsx") filename = os.path.relpath(filename) if os.path.isfile(filename): self.filename = filename with warnings.catch_warnings(): warnings.filterwarnings("ignore", "Workbook contains no default style", UserWarning) self.workbook = xl.load_workbook(self.filename,data_only=True) self.sheetNames = self.workbook.sheetnames logger.debug(f"Sheet names from default database {self.sheetNames}") # Close the work book while it is not in use # workbook.close() else: self.filename = None self.sheetNames = None logger.error(f"Error: MaterialsDataBase filename not valid {filename}") self.cache = {} logger.debug("Finished:: initialise") return
[docs] def get_file_name(self): """Return the filename. Parameters ---------- None Returns ------- str The filename. """ return self.filename
[docs] def valid(self): """Test to see if the spreadsheet is a valid materials database. Parameters ---------- None Returns ------- bool True if the spreadshee is 'valid' Notes ----- None """ result = False if "Information" in self.sheetNames[0]: result = True return result
[docs] def get_sheet_names(self): """Return a list of the sheetnames in the database. As well as the sheets in the database, there are some default materials which will be added to the list of materials and which are provided internally by this module. Parameters ---------- None Returns ------- list A list of the sheet names present in the database. """ # First take a copy of the sheetnames ignoring the first (Information) fullList = [] if self.sheetNames is not None: fullList = self.sheetNames[1:].copy() # Append any in-built materials # This list is taken from the original powder code before version 8.0 if "air" not in fullList: fullList.append("air") if "vacuum" not in fullList: fullList.append("vacuum") if "ptfe" not in fullList: fullList.append("ptfe") if "ldpe" not in fullList: fullList.append("ldpe") if "mdpe" not in fullList: fullList.append("mdpe") if "kbr" not in fullList: fullList.append("kbr") if "nujol" not in fullList: fullList.append("nujol") if "none" not in fullList: fullList.append("none") logger.debug(f"get_sheet_names:: {fullList}") return sorted(fullList, key=lambda s: s.casefold())
[docs] def get_material(self,sheet): """Return a material object based on the data in sheet (an excel sheet). If one of the following is requested: air, vacuum, ptfe, ldpe, mdpe, kbr, nujol, none, then the material is created even if it is not in the database. Parameters ---------- sheet : Excel sheet The excel sheet containing the material data. Returns ------- Material object The material object created from the excel sheet data. """ logger.debug(f"get_material:: {sheet}") # Lets see if the material is in the cache if sheet in self.cache: logger.debug("get_material:: using the cache") return self.cache[sheet] # Define a set of back-up materials that the program can use even if the sheet name is not in the spreadsheet if self.sheetNames is None or sheet not in self.sheetNames: if sheet == "air": material = Constant("air",permittivity=1.0,density=0.001225) elif sheet == "vacuum": material = Constant("vacuum",permittivity=1.0,density=0.0) elif sheet == "ptfe": material = Constant("ptfe",permittivity=2.0,density=2.2) elif sheet == "ldpe": material = Constant("ldpe",permittivity=2.25,density=0.925) elif sheet == "mdpe": material = Constant("mdpe",permittivity=2.25,density=0.933) elif sheet == "kbr": material = Constant("kbr",permittivity=2.25,density=2.75) elif sheet == "nujol": material = Constant("nujol",permittivity=2.155,density=0.838) elif sheet == "none": material = NoMatrix() else: logger.error(f"Error in get_material sheet {sheet} not in self.sheetNames {self.sheetNames}") material = Constant("vacuum",permittivity=1.0,density=0.0) return material # Carry on with the spreadsheet # workbook = xl.load_workbook(self.filename,data_only=True) worksheet = self.workbook[sheet] unitCell = None optical_permittivity = None avector = bvector = cvector = None a = b = c = alpha = beta = gamma = None for i in range(20): cell1 = "G"+str(i+1) cell2 = "H"+str(i+1) token = worksheet[cell1].value if token is not None: token = token.lower() if "entry" in token: entry = worksheet[cell2].value.lower() elif "density" in token: density = float(worksheet[cell2].value) elif "optical_permittivity" in token: optical_permittivity = float(worksheet[cell2].value) elif "a_vector" in token: avector = [ float(cell.value) for cell in [ worksheet["I"+str(i+1)], worksheet["J"+str(i+1)], worksheet["K"+str(i+1)] ] ] elif "b_vector" in token: bvector = [ float(cell.value) for cell in [ worksheet["I"+str(i+1)], worksheet["J"+str(i+1)], worksheet["K"+str(i+1)] ] ] elif "c_vector" in token: cvector = [ float(cell.value) for cell in [ worksheet["I"+str(i+1)], worksheet["J"+str(i+1)], worksheet["K"+str(i+1)] ] ] elif token == "a:": a = float(worksheet[cell2].value) elif token == "b:": b = float(worksheet[cell2].value) elif token == "c:": c = float(worksheet[cell2].value) elif "alpha" in token: alpha = float(worksheet[cell2].value) elif "beta" in token: beta = float(worksheet[cell2].value) elif "gamma" in token: gamma = float(worksheet[cell2].value) if avector is not None and bvector is not None and cvector is not None: unitCell = UnitCell(a=avector,b=bvector,c=cvector) elif a is not None and b is not None and c is not None and alpha is not None and beta is not None and gamma is not None: unitCell = UnitCell(a=a,b=b,c=c,alpha=alpha,beta=beta,gamma=gamma) # Process the entry type if "constant" in entry and "refractive" in entry: material = self.read_constant_refractive_index(sheet,worksheet,density) elif "constant" in entry and ("permitt" in entry or "dielec" in entry): material = self.read_constant_permittivity(sheet,worksheet,density) elif "tabulated" in entry and "refractive" in entry: material = self.read_tabulated_refractive_index(sheet,worksheet,density) elif "tabulated" in entry and "spec" in entry: material = self.read_tabulated_spectroscopy(sheet,worksheet,density) elif "tabulated" in entry and ("permitt" in entry or "dielec" in entry): material = self.read_tabulated_permittivity(sheet,worksheet,density) elif "lorentz" in entry and "drude" in entry: material = self.read_lorentz_drude(sheet,worksheet,density,unitCell) elif "fpsq" in entry: material = self.read_fpsq(sheet,worksheet,density,unitCell) elif "sellmeier" in entry: material = self.read_sellmeier(sheet,worksheet,density,unitCell) # # Add the optical permittivity material.optical_permittivity = optical_permittivity # Close the work book # workbook.close() # Add the material to the cache self.cache[sheet] = material return material
[docs] def read_constant_refractive_index(self,sheet,worksheet,density): """Read constant refractive index from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet. density : float The density of the material. Returns ------- None """ # Constant refractive index n = float(worksheet["C2"].value) k = float(worksheet["D2"].value) nk = complex(n, k) permittivity = Calculator.calculate_permittivity(nk) logger.debug(f"Constant refractive:: {nk} {permittivity} {density}") return Constant(sheet,permittivity=permittivity,density=density)
[docs] def read_constant_permittivity(self,sheet,worksheet,density): """Read constant permittivity data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet instance. density : float The density of the material. Returns ------- None """ # Constant permittivity eps_r = float(worksheet["C2"].value) eps_i = float(worksheet["D2"].value) permittivity = complex(eps_r, eps_i) logger.debug(f"Constant permittivity:: {permittivity} {density}") return Constant(sheet,permittivity=permittivity,density=density)
[docs] def read_tabulated_refractive_index(self,sheet,worksheet,density): """Read tabulated refractive index data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet. density : float The density of the material. Returns ------- None """ # Tabulated refractive index permittivities = [] vs_cm1 = [] for a, c, d in zip(worksheet["A"][1:] ,worksheet["C"][1:] , worksheet["D"][1:]): if a.value is None or c.value is None or d.value is None: break try: v = float(a.value) n = float(c.value) k = float(d.value) nk = complex(n, k) permittivity = Calculator.calculate_permittivity(nk) permittivities.append(permittivity) vs_cm1.append(v) except (ValueError, TypeError): logger.error(f"Error in Tabulated: {a.value} {c.value} {d.value}") return Tabulated(sheet,vs_cm1,permittivities=permittivities,density=density)
[docs] def read_tabulated_spectroscopy(self,sheet,worksheet,density): """Read tabulated refractive index data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet. density : float The density of the material. Returns ------- None """ # Tabulated refractive index + absorption (in cm^-1) permittivities = [] vs_cm1 = [] for a, c, d in zip(worksheet["A"][1:] ,worksheet["C"][1:] , worksheet["D"][1:]): if a.value is None or c.value is None or d.value is None: break try: v = float(a.value) n = float(c.value) a = float(d.value) k = a /(v * 4 * np.pi * math.log10(math.e)) nk = complex(n, k) permittivity = Calculator.calculate_permittivity(nk) permittivities.append(permittivity) vs_cm1.append(v) except (ValueError, TypeError): logger.error(f"Error in Tabulated: {a.value} {c.value} {d.value}") #return permittivities, vs_cm1 return Tabulated(sheet,vs_cm1,permittivities=permittivities,density=density)
[docs] def read_tabulated_permittivity(self,sheet,worksheet,density): """Read tabulated permittivity data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet. density : float The density of the material. Returns ------- None """ # Tabulated permittivity permittivities = [] vs_cm1 = [] for a, c, d in zip(worksheet["A"][1:] ,worksheet["C"][1:] , worksheet["D"][1:]): if a.value is None or c.value is None or d.value is None: break v = float(a.value) eps_r = float(c.value) eps_i = float(d.value) permittivity = complex(eps_r, eps_i) permittivities.append(permittivity) vs_cm1.append(v) return Tabulated(sheet,vs_cm1,permittivities=permittivities,density=density)
[docs] def read_lorentz_drude(self,sheet,worksheet,density,unitCell): """Read Drude-Lorentz data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet. density : float The density of the material. unitCell : object The unit cell. Returns ------- None """ # Lorentz-Drude model for permittivity epsilon_infinity = np.zeros( (3,3) ) omegas = [[], [], []] strengths = [[], [], []] gammas = [[], [], []] for a, b, c, d, e in zip(worksheet["A"][1:] ,worksheet["B"][1:] , worksheet["C"][1:], worksheet["D"][1:], worksheet["E"][1:]) : try: if a.value is not None: direction = a.value index = ["xx","yy","zz"].index(direction) if b.value is not None: epsilon_infinity[[index],[index]] = float(b.value) if c.value is not None: omegas[index].append(float(c.value)) if d.value is not None: strengths[index].append(float(d.value)) if e.value is not None: gammas[index].append(float(e.value)) except (ValueError, TypeError): logger.error(f"Error in Lorentz-Drude: {a.value} {b.value} {c.value} {d.value} {e.value}") return None return DrudeLorentz(sheet,epsilon_infinity,omegas,strengths,gammas,density=density,cell=unitCell)
[docs] def read_fpsq(self,sheet,worksheet,density,unitCell): """Read FPSQ data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The actual worksheet object. density : float The density of the material. unitCell : object The unit cell. Returns ------- None """ # FPSQ model for permittivity epsilon_infinity = np.zeros( (3,3) ) omega_tos = [[], [], []] gamma_tos = [[], [], []] omega_los = [[], [], []] gamma_los = [[], [], []] for a, b, c, d, e, f in zip(worksheet["A"][1:] ,worksheet["B"][1:] , worksheet["C"][1:], worksheet["D"][1:], worksheet["E"][1:], worksheet["F"][1:]) : try: if a.value is not None: direction = a.value index = ["xx","yy","zz"].index(direction) if b.value is not None: epsilon_infinity[[index],[index]] = float(b.value) if c.value is not None: omega_tos[index].append(float(c.value)) if d.value is not None: gamma_tos[index].append(float(d.value)) if e.value is not None: omega_los[index].append(float(e.value)) if f.value is not None: gamma_los[index].append(float(f.value)) except (ValueError, TypeError): logger.error(f"Error in FPSQ: {a.value} {b.value} {c.value} {d.value} {e.value} {f.value}") return None return FPSQ(sheet,epsilon_infinity,omega_tos,gamma_tos,omega_los,gamma_los,density=density,cell=unitCell)
[docs] def read_sellmeier(self,sheet,worksheet,density,unitCell): """Read Sellmeier data from the spreadsheet. Parameters ---------- sheet : str The worksheet name. worksheet : worksheet The worksheet. density : float The density of the material. unitCell : object The unit cell. Returns ------- None """ # Sellmeier model for refractive index Bs = [] Cs = [] for b, c in zip(worksheet["A"][1:] , worksheet["B"][1:] ) : try: if b.value is not None: Bs.append(float(b.value)) if c.value is not None: Cs.append(float(c.value)) except (ValueError, TypeError): logger.error(f"Error in Sellmeier: {b.value} {c.value}") return None return Sellmeier(sheet,Bs,Cs,density=density,cell=unitCell)
[docs] class _ClampedPermittivity: """Picklable wrapper that clamps a permittivity function above a frequency threshold. Used by :meth:`Material.get_permittivity_function` so the returned callable can be sent to multiprocessing pool workers via pickle. """ def __init__(self, inner, freq_max_cm1, optical, is_scalar): self.inner = inner self.freq_max_cm1 = freq_max_cm1 self.optical = optical self.is_scalar = is_scalar
[docs] def __call__(self, v): if v > self.freq_max_cm1: if self.is_scalar: return complex(self.optical) return np.array(self.optical, dtype=np.cdouble) return self.inner(v)
[docs] class Material: """A class for representing materials with properties like name, density, permittivity, and unit cell. The Material class also contains the permittivity object for the material. The permittivity object is an instance of :class:`~PDielec.DielectricFunction.DielectricFunction` or one its children. The permittivity object is responsible for calculating the permittivity at the given frequency. The subclasses which inherit from the Material class are: Constant, External, DrudeLorentz, FPSQ, Sellmeier, and Tabulated. Each subclass has an initialisation routine which instantiates the permittivity object of the appropriate type for the material. The relationship between the Material subclass and the DielectricFunction subclass of the permittivity object is shown below. +---------------------------+-------------------------------------------------------------+ | Material subclass | DielectricFunction subclass | +===========================+=============================================================+ | :class:`Constant` | :class:`~PDielec.DielectricFunction.Constant` | +---------------------------+-------------------------------------------------------------+ | :class:`NoMatrix` | :class:`~PDielec.DielectricFunction.ConstantScalar` (1.0) | | | placeholder; bypasses EMT entirely when used as matrix. | +---------------------------+-------------------------------------------------------------+ | :class:`External` | This class is passed a permittivity object which has been | | | defined externally | +---------------------------+-------------------------------------------------------------+ | :class:`DrudeLorentz` | :class:`~PDielec.DielectricFunction.DrudeLorentz` | +---------------------------+-------------------------------------------------------------+ | :class:`FPSQ` | :class:`~PDielec.DielectricFunction.FPSQ` | +---------------------------+-------------------------------------------------------------+ | :class:`Sellmeier` | :class:`~PDielec.DielectricFunction.Sellmeier` | +---------------------------+-------------------------------------------------------------+ | :class:`Tabulated` | :class:`~PDielec.DielectricFunction.TabulateScalar` | | | :class:`~PDielec.DielectricFunction.Tabulate3` | | | :class:`~PDielec.DielectricFunction.Tabulate3` | | | :class:`~PDielec.DielectricFunction.Tabulate6` | +---------------------------+-------------------------------------------------------------+ Parameters ---------- name : str The name of the material. optical_permittivity : float, optional The optical permittivity of the material density : float, optional The density of the material. If not provided and a cell is given, it will be calculated based on the cell. permittivity_object : :class:`~PDielec.DielectricFunction.DielectricFunction`, optional An object representing the dielectric function of the material. This is intended to be passed by classes that inherit from Material, and it should contain methods for calculating scalar/tensor permittivity. (see :class:`~PDielec.DielectricFunction.DielectricFunction` and its sub-classes) cell : :class:`~PDielec.UnitCell.UnitCell`, optional An object representing the unit cell of the material. If provided without a density, the density will be calculated from this cell. (See :class:`~PDielec.UnitCell.UnitCell`) Attributes ---------- density : float or None The density of the material, which may be calculated based on the cell if not provided initially. optical_permittivity : float or None The scalar optical permittivity of the material cell : Cell or None The unit cell of the material if provided. name : str The name of the material. type : str A string indicating the type of the object. Defaults to 'Base Class' for the base Material class. permittivity_object : DielectricFunction or None An object to handle the permittivity calculations for the material. Methods ------- get_name() Returns the name of the material. get_information() Returns information about the material, including its type and, if applicable, its permittivity frequency range. get_sigmas() If the material has a lorentzian dielectric this routine returns the sigma parameters set_sigmas() If the material has a lorentzian dielectric this routine sets the sigma parameters get_frequencies() If the material has a lorentzian dielectric this routine returns the frequencies set_frequencies() If the material has a lorentzian dielectric this routine sets the frequencies get_oscillator_strengths() If the material has a lorentzian dielectric this routine returns the oscillator strengths set_oscillator_strengths() If the material has a lorentzian dielectric this routine sets the oscillator strengths print() Prints information about the material, such as its name, density, type, and permittivity details. is_scalar() Checks and returns True if the material’s permittivity is scalar. is_tensor() Checks and returns True if the material’s permittivity is tensor. get_permittivity_object() Returns the permittivity_object of the material. get_permittivity_function() Returns the permittivity function from the permittivity_object. get_density() Returns the density of the material. set_cell(cell) Sets the cell of the material and updates the density if it was initially None. get_cell() Returns the cell of the material. set_density(value) Sets the density of the material. set_epsilon_infinity(eps) Sets the epsilon infinity of the material set_permittivity_object(permittivity_object) Sets the permittivity_object for the material. """ def __init__(self, name, density=None, permittivity_object=None, cell=None, optical_permittivity=None): """Initialise a material with the following parameters. Parameters ---------- name : str The name of the material. optical_permittivity : float, optional The optical permittivity of the material Note this is not the same as epsilon_infinity which is only used to define the dielectric function If this is None, the dielectric function is asked for the optical permittivity density : float, optional The density of the material. If not provided and a cell is given, it will be calculated based on the cell. permittivity_object : DielectricFunction, optional An object representing the dielectric function of the material. This is intended to be passed by classes that inherit from Material, and it should contain methods for calculating scalar/tensor permittivity. cell : unitCell, optional An object representing the unit cell of the material. If provided without a density, the density will be calculated from this cell. Notes ----- The material object is created from the name, density, optical_permittivity and unit cell. The permittivity object is specifically created by the children of Material, indicating it's a derived property or capability not initialized directly by the Material's constructor but through some other process or method within the child classes. """ self.density = density self.optical_permittivity = optical_permittivity self.cell = cell self.name = name self.type = "Base Class" self.permittivity_object = permittivity_object if self.density is None and self.cell is not None: self.density = self.cell.get_density("cm")
[docs] def get_name(self): """Get the name attribute of the object. Parameters ---------- None Returns ------- str The name attribute of the object. """ return self.name
[docs] def get_information(self): """Return information about the material. Parameters ---------- None Returns ------- str A description of the material. """ result = self.type if "Tabulate" in self.type: low = self.permittivity_object.get_lowest_frequency() high = self.permittivity_object.get_highest_frequency() result += f" freq range {low:.0f}-{high:.0f}" # + ' value at 0 {}'.format(self.permittivity_object.function()(0)) # result += ' value at 0 {}'.format(self.permittivity_object.function()(0)) return result
[docs] def print(self): """Print information about the material. Parameters ---------- None Returns ------- None """ print("Material name:",self.name) print("Material density:",self.density) print("Material type:",self.type) print("Material optical permittivity:",self.optical_permittivity) print("Material is scalar?:",self.is_scalar()) print("Material is tensor?:",self.is_tensor()) print("Material permittivity:",self.get_information()) if self.cell is not None: print("Material unit cell") self.cell.print() return
[docs] def is_scalar(self): """Return true if the material returns a scalar permittivity. Parameters ---------- None Returns ------- bool True if the material returns a scalar permittivity, False otherwise. """ return self.permittivity_object.is_scalar()
[docs] def is_tensor(self): """Return true if the material returns a tensor permittivity. Parameters ---------- None Returns ------- bool True if the material returns a tensor permittivity, False otherwise. """ return self.permittivity_object.is_tensor()
[docs] def set_permittivity_object(self,permittivity_object): """Set the permittivity object. Parameters ---------- permittivity_object : a permittivity object (dielectric function object) The permittivity object is used to calculate the permittivity of the material Returns ------- None """ self.permittivity_object = permittivity_object return
[docs] def get_permittivity_object(self): """Return the permittivity object. Parameters ---------- None Returns ------- permittivity_object Return the permittivity object (dielectric function object) """ return self.permittivity_object
[docs] def get_permittivity_function(self): """Return the permittivity function. Parameters ---------- None Returns ------- permittivityObjectFunction Return the permittivity object function. If the material has an ``optical_permittivity`` and the underlying permittivity object has a finite tabulated frequency range, the returned function clamps to the ``optical_permittivity`` value for frequencies above the highest tabulated frequency. This prevents unphysical extrapolation of IR dielectric models to optical (laser) frequencies. """ inner = self.permittivity_object.function() # Only clamp when we have an explicit optical_permittivity and the # underlying model has a finite tabulated range (vs_cm1 is an array). if self.optical_permittivity is None: return inner vs = self.permittivity_object.vs_cm1 if not isinstance(vs, np.ndarray) or vs.size == 0: return inner freq_max_cm1 = float(np.max(vs)) optical = self.get_optical_permittivity() is_scalar = self.is_scalar() return _ClampedPermittivity(inner, freq_max_cm1, optical, is_scalar)
[docs] def get_optical_permittivity(self): """Return the optical (high-frequency) permittivity of this material. If the material has an optical permittivity specified it is returned. Otherwise it delegates to the underlying permittivity object's :meth:`~PDielec.DielectricFunction.DielectricFunction.optical_permittivity` method. For tensor materials this returns a 3×3 real tensor; for scalar materials it returns a float. Returns ------- float or ndarray The optical permittivity. """ if self.optical_permittivity is None: return self.permittivity_object.optical_permittivity() optical = np.asarray(self.optical_permittivity) if optical.ndim == 0: optical = float(np.real(optical)) if self.is_scalar(): return optical return optical * np.eye(3) return optical
[docs] def set_frequencies(self,frequencies): """Set the frequencies for a Lorentzian permittivity. Parameters ---------- frequencies : 1D array of floats The frequencies for a Drude-Lorentzian permittivity in cm-1 Returns ------- None """ self.permittivity_object.set_frequencies(frequencies) return
[docs] def get_frequencies(self): """Get the frequencies for a Lorentzian permittivity. Parameters ---------- None Returns ------- 1d array of floats Returns the frequencies for a Lorentzian function in cm-1 """ return self.permittivity_object.get_frequencies()
[docs] def set_oscillator_strengths(self,strengths): """Set the oscillator strengths for a Lorentzian permittivity. Parameters ---------- strengths : a 3x3 array of floats for each frequency The oscillator strengths for a Lorentzian permittivity function in cm-1 Returns ------- None """ self.permittivity_object.set_oscillator_strengths(strengths) return
[docs] def get_oscillator_strengths(self): """Get the oscillator strengths for a Lorentzian permittivity. The oscillator strength of each transition is a 3x3 matrix Parameters ---------- None Returns ------- list of 3x3 array of floats Returns the oscillator strengths for a Lorentzian permittivity function in cm-1 """ return self.permittivity_object.get_oscillator_strengths()
[docs] def set_sigmas(self,sigmas): """Set the sigma parameters for a Lorentzian permittivity. Parameters ---------- sigmas : 1D array of floats The sigma parameters for a Lorentzian permittivity function in cm-1 Returns ------- None """ self.permittivity_object.set_sigmas(sigmas) return
[docs] def get_sigmas(self): """Get the sigma parameters for a Lorentzian permittivity. Parameters ---------- None Returns ------- 1d array of floats Returns the sigma parameters for a Lorentz permittivity function in cm-1 """ return self.permittivity_object.get_sigmas()
[docs] def set_density(self, value): """Set the density. Parameters ---------- value : float The value of the density Returns ------- None """ self.density = value return
[docs] def get_density(self): """Return the density. Parameters ---------- None Returns ------- self.density """ return self.density
[docs] def set_cell(self, cell): """Set the unit cell. Parameters ---------- cell : a unit cell Set the unit cell of the material Returns ------- None """ self.cell = cell if self.density is None and self.cell is not None: self.density = self.cell.calculate_density() return
[docs] def get_cell(self): """Return the cell. Parameters ---------- None Returns ------- self.cell """ return self.cell
[docs] class Constant(Material): """A class representing a material with constant scalar permittivity, inheriting from the `Material` class. Attributes ---------- type : str The type of material, set to 'Constant permittivity'. Methods ------- Inherits methods from the `Material` class. """ def __init__(self, name, permittivity=None, density=None, cell=None): """Create an instance of a material with a constant scalar permittivity. Permittivity is the value of the permittivity and can be complex. Parameters ---------- name : str The name of the material. permittivity : complex The permittivity value. It can be a complex number. density : float The density of the material in g/ml. cell : unitCell The unit cell. """ super().__init__(name, density=density, permittivity_object=DielectricFunction.ConstantScalar(permittivity), cell=cell) self.type = "Constant permittivity"
[docs] class NoMatrix(Material): """A sentinel material representing no support matrix. When selected as the support matrix, calculations bypass effective medium theory entirely. Infrared spectra are computed directly from the isotropic average of the DFT crystal permittivity tensor. Raman spectra use the raw DFT Raman tensors with no local-field (internal-field) correction and no particle-shape frequency shift. Attributes ---------- type : str Set to 'No matrix (DFT only)'. """ def __init__(self): """Create a NoMatrix material. The permittivity is set to 1.0 as a placeholder; it is not used in any actual calculation when this material is active. """ super().__init__("none", density=0.0, permittivity_object=DielectricFunction.ConstantScalar(1.0)) self.type = "No matrix (DFT only)"
[docs] class External(Material): """A class for representing materials with externally specified permittivity. This class inherits from the `Material` class and is used to define materials where the permittivity is specified externally, rather than calculated or predefined. Permittivity can be a complex value indicating both the real and imaginary parts. """ def __init__(self, name, permittivity_object=None, density=None, cell=None): """Create an instance of a material which has the permittivity object specified externally. The permittivity can be a complex number. Parameters ---------- name : str The name of the material. permittivity_object : complex The permittivity value, which can be a complex number. density : float The density of the material in grams per milliliter (g/ml). cell : unitCell The unit cell of the material. Returns ------- object An instance of the material with the specified permittivity object. """ super().__init__(name, density=density, permittivity_object=permittivity_object, cell=cell) self.type = "External permittivity"
[docs] class DrudeLorentz(Material): """A subclass representing a material with a Lorentz-Drude model permittivity. Parameters ---------- name : str The name of the material. epsinf : array_like Epsilon infinity, either a 3x3 list or a 3x3 array representing the static dielectric constant. omegas : list The transverse optical (TO) frequencies. strengths : list The oscillator strengths for each resonance. gammas : list The damping (or broadening) factors for each resonance. density : float, optional The density of the material in grams per milliliter (g/ml). Default is None. cell : unitCell, optional The unit cell of the material. Default is None. Notes ----- The Drude-Lorentz model is used to calculate the permittivity of the material by considering the contributions from both free electrons (Drude) and bound electrons (Lorentz). This class requires specifying the infinite frequency dielectric constant (`epsinf`), the transverse optical frequencies (`omegas`), the oscillator strengths (`strengths`), and the damping factors (`gammas`) for each resonance in the material. Examples -------- >>> drude_lorentz_material = DrudeLorentz("Gold", [[1, 0, 0], [0, 1, 0], [0, 0, 1]], ... [0.5, 1.0], [1.0, 2.0], [0.2, 0.1], ... density=19.3) This represents a Drude-Lorentz material with the name "Gold", an isotropic epsilon infinity, two resonances with specified frequencies, strengths, and damping factors, and a density of 19.3 g/ml. """ def __init__(self, name,epsinf,omegas,strengths,gammas,density=None,cell=None): """Create an instance of a material with a Lorentz Drude model permittivity. Parameters ---------- name : str The name of the material. epsinf : list or array Epsilon infinity either a 3x3 list or a 3x3 array. omegas : list The Transverse Optical (TO) frequencies. strengths : list The absorption strengths. gammas : list The absorption widths. density : float The density of the material in g/ml. cell : unitCell The unit cell of the material. """ epsilon_infinity = np.array(epsinf) permittivity_object = DielectricFunction.DrudeLorentz( omegas, strengths, gammas) permittivity_object.set_epsilon_infinity(epsilon_infinity) super().__init__(name, density=density, permittivity_object=permittivity_object,cell=cell) self.type = "Drude-Lorentz"
[docs] class FPSQ(Material): """Class representing a material with a FPSQ model for permittivity. Parameters ---------- name : str The name of the material. epsinf : array_like Epsilon infinity (eps0), either a 3x3 list or a 3x3 array representing the dielectric constant at infinite frequency. omega_tos : list The transverse optical (TO) frequencies. gamma_tos : list The TO absorption widths. omega_los : list The longitudinal optical (LO) frequencies. gamma_los : list The LO absorption widths. density : float, optional The density of the material in grams per milliliter (g/ml). cell : unitCell, optional The unit cell of the material. Notes ----- The FPSQ (fitted phonon simple quantum) model is used to describe the permittivity of the material. This model is based on the harmonic oscillator model and describes the permittivity as a function of frequency. """ def __init__(self, name,epsinf,omega_tos,gamma_tos,omega_los,gamma_los,density=None,cell=None): """Create an instance of a material with an FPSQ model permittivity. Parameters ---------- name : str The name of the material. epsinf : list or ndarray Epsilon infinity (ε∞), either a 3x3 list or a 3x3 array. omega_tos : list The transverse optical (TO) frequencies. gamma_tos : list The TO absorption widths. omega_los : list The longitudinal optical (LO) frequencies. gamma_los : list The LO absorption widths. density : float Density in g/ml. cell : unitCell The unit cell. """ epsilon_infinity = np.array(epsinf) permittivity_object = DielectricFunction.FPSQ( omega_tos, gamma_tos, omega_los, gamma_los) permittivity_object.set_epsilon_infinity(epsilon_infinity) super().__init__(name, density=density, permittivity_object=permittivity_object,cell=cell) self.type = "FPSQ"
[docs] class Sellmeier(Material): """A class to define materials using the Sellmeier model for permittivity. Parameters ---------- name : str The name of the material. Bs : list or array_like The B parameters (coefficients) in the Sellmeier equation. Cs : list or array_like The C parameters (coefficients) in the Sellmeier equation. density : float, optional The density of the material in g/ml. Default is None. cell : unitCell, optional The unit cell of the material. Default is None. Attributes ---------- type : str The type of the material, which is 'Sellmeier' for instances of this class. Methods ------- __init__(self, name, Bs, Cs, density=None, cell=None) Initializes a Sellmeier material with specified parameters. """ def __init__(self, name,Bs,Cs,density=None,cell=None): """Create an instance of a material with a Sellmeier model permittivity. Permittivity is the value of the permittivity and should be real for the Sellmeier model. The required parameters are: Parameters ---------- name : str The name of the material. Bs : list The B parameters of the Sellmeier equation. Cs : list The C parameters of the Sellmeier equation. density : float Density in g/ml. cell : unitCell The unit cell. """ permittivity_object = DielectricFunction.Sellmeier( Bs, Cs) super().__init__(name, density=density, permittivity_object=permittivity_object,cell=cell) self.type = "Sellmeier"
[docs] class Tabulated(Material): """A class for materials with tabulated permittivities. Parameters ---------- name : str The name of the material. vs_cm1 : list or None, optional The list of tabulated frequencies in cm-1. Defaults to None. permittivities : array-like or None, optional The permittivities, either as a single vector (n,) or a tensor (3,n) or (6,n) for more complex materials. Defaults to None. density : float or None, optional The density of the material in g/ml. Defaults to None. cell : unitCell or None, optional The unit cell of the material. Defaults to None. Notes ----- - This class is designed to handle materials with a constant permittivity as well as those requiring more complex permittivity tensors. - The permittivity can be defined using either a scalar for simple materials or tensors for materials that require a support matrix. - The constructor converts the input lists of frequencies (`vs_cm1`) and permittivities into numpy arrays, and then generates the appropriate permittivity object depending on the complexity of the material's permittivities. Examples -------- >>> material1 = Tabulated("Quartz", vs_cm1=[500, 1000, 1500], permittivities=[2.1, 2.3, 2.5], density=2.65) >>> material2 = Tabulated("Synthetic", vs_cm1=[200, 400, 600], permittivities=[[2.1, 2.3, 2.5], [2.4, 2.6, 2.8], [3.0, 3.2, 3.4]], density=1.5) """ def __init__(self, name, vs_cm1=None, permittivities=None, density=None, cell=None): """Create an instance of a material with a constant permittivity. Permittivity is the value of the permittivity and can be complex. The returned permittivity_object can generate either a scalar or a tensor. For defining a support matrix material, a scalar is used. Parameters ---------- name : str The name of the material. vs_cm1 : list The list of tabulated frequencies in cm-1. permittivities : array_like The permittivities, either a single (n) vector or a (3,n) vector. density : float Density in g/ml. cell : unitCell The unit cell. """ vs = np.array(vs_cm1) eps = np.array(permittivities) if len(np.shape(eps)) == 2: m,n = np.shape(eps) if m == 3: permittivity_object = DielectricFunction.Tabulate3(vs,eps[0], eps[1], eps[2]) elif m== 6: permittivity_object = DielectricFunction.Tabulate6(vs,eps[0], eps[1], eps[2], eps[3], eps[4], eps[5]) else: logger.error("Error in Tabulated, shape of parameters is wrong") else: permittivity_object = DielectricFunction.TabulateScalar(vs,eps) super().__init__(name, density=density, permittivity_object=permittivity_object,cell=cell) self.type = "Tabulated permittivity"
[docs] def set_epsilon_infinity(self,eps): """Set the value of epsilon infinity for the material. Parameters ---------- eps : float or 3x3 np array The epsilon infinity tensor. If a single float then an isotropic 3x3 np array is created Returns ------- None """ eps = eps*np.eye(3) if isinstance(eps,float) else np.array(eps) self.permittivity_object.set_epsilon_infinity(eps)